MBI staff member
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Dr. Arnaud Rouzee

rouzee@mbi-berlin.de

+49 30 6392 1240

Research scientist

Project Coordinator: 2.3 "Time-resolved XUV science"

Member of Projects: 2.2

 

Research Topic


Short introduction:


The recent develoment of ultrashort bursts of short wavelength radiation opens new routes to image molecules and their dynamics with unprecedent spatial and temporal resolution. In our group, we are implementing time-resolved XUV and X-ray imaging techniques in extended systems from polyatomic molecules to clusters to explore the details of multielectron dynamics and electron-nuclear couplings.

"Strong field ionization of atoms and molecules"


"Ultrafast XUV/X-ray & photoelectron imaging"


"Multiphoton XUV and X-ray ionization dynamics"


"Femtosecond and attosecond molecular dynamics"



 



Curriculum vitae


  • 2014-present: Permanent staff scientist
    Project coordinator : 2.3 time-resolved XUV science
    Max-Born-Institute, Berlin, Germany.
  • 2011-2014: Postdoctoral Fellow II Max-Born-Institute, Berlin, Germany.
  • 2010-2011: Guest scientist Max-Born-Institute, Berlin, Germany.
  • 2007-2011: Postdoctoral Fellow I FOM institute, AMOLF
  • 2004-2007: Lecturer French CIES Monitor Dijon University
  • 2004-2007: Ph.D. Thesis: "Laser-induced molecular alignment of asymmetric top molecules", Dijon University

 

Research Highlights


Publications


Publications at MBI



Full List of publications :

  • Autoionization following nanoplasma formation in atomic and molecular clusters, B. Schuette, J. Lahl, T. Oelze, M. Krikunova, M. J. J. Vrakking, A. Rouzee, European Physical Journal D, 70, 115, (2016).

  • Femtosecond and nanometer visualization of structural dynamics in superheated nanoparticles, T. Ghorkover, et al., Nature Photonics, 10, 93, (2016).

  • Ionization avalanching in clusters ignited by extreme-ultraviolet driven seed electrons, B. Schuette, M. Arbeiter, A. Mermillod-Blondin, M. J. J. Vrakking, A. Rouzee, T. Fennel, Phys. Rev. Lett., 116, 033001, (2016).

  • Bright attosecond soft X-ray pulse trains by transient phase-matching in two-color high-order harmonic generation, B. Schuette, P. Weber, K. Kovacs, E. Balogh, B. Major, V. Tosa, S. Han, M. J. J. Vrakking, A. Rouzee, Optics express, 23, 33947, (2015).

  • Initial electronic coherence in molecular dissociation induced by an attosecond pulse, Lukas Medisauskas, S. Patchkovskii, A. Harvey, D. S. Bramdila, C. Neidel, J. Klei, A. Rouzee, M. J. J. Vrakking, M. Y. Ivanov, Phys. Rev. A., 92, 053403, (2015).

  • Observation of correlated electronic decay in expanding clusters triggered by near-infrared fields, B. Schuette, M. Arbeiter, Th. Fennel, G. Jabbari, A. Kuleff, M. J. J. Vrakking, A. Rouzee, Nature communication, 6, 8596, (2015).

  • Real time fragmentation dynamics of clusters ionized by extreme ultraviolet pulses, B. Schuette, T. Oelze, M. Krikunova, M. Arbeiter, T. Fennel, M. J. J. Vrakking, and A. Rouzee, J. Phys. B, 48, 185101, (2015).

  • XUV excitation followed by ultrafast non-adiabatic relaxation in PAH molecules as a femto-astrochemistry experiment, A. Marciniak, V. Despre, T. Barillot, A. Rouzee, M. Galbraith, J. Klei, CH. Yang, C. Smeenk, V. Loriot, S. N. Reddy, A. G. G. M. Tielens, S. Mahapatra, A. I. Kuleff, M. J. J. Vrakking, F. Lepine, Nature Communication, 6, 7909, (2015).

  • Recombination and fragmentation dynamics of clusters in intense extreme-ultraviolet and near-infrared fields, B. Schuette, T. Oelze, M. Krikunova, M. Arbeiter, T. Fennel, M. J. J. Vrakking, A. Rouzee, New J. of Phys., 17, 033043, (2015).

  • Efficient autoionization following intense laser-clusters interaction, B. Schuette, J. Lahl, T. Oelze, M. Krikunova, M. J. J. Vrakking, A. Rouzee, Phys. Rev. Lett., 114, 123002, (2015).

  • Attosecond hole migration in Benzene molecules nuclear motion, V. Despre, A. Marciniak, V. Loriot, M.C.E. Galbraith, A. Rouzee, M.J.J. Vrakking, F. Lepine, A. I. Kuleff, J. Phys. Chem. Lett., 6, 426, (2015).

  • Probing the structure and dynamics of molecular clusters using molecular wavepackets, G. Galinis, C. Cacho, R. T. Chapman, A. M. Ellis, M. Lewerenz, L.G.M. Luna, R.S. Minns, M. Mladenic, A. Rouzee, E. Springate, I.C.E. Turcu, M.J. Watkins, K. von Haeften, Phys. Rev. Lett., 113, 043004, (2014).

  • Femtosecond X-ray photoelectron diffraction on gas-phase dibromobenzene molecules, D. Rolles et al., J. Phys. B, 47, 124035, (2014).

  • Imaging the electronic structure of valence orbital in the XUV ionization of aligned molecules, A. Rouzee, A. G. Harvey, K. Kelkensberg, D. Brambila, W. K. Siu, G. Gademann, O. Smirnova, M. J. J. Vrakking, J. Phys B, 47, 124017, (2014).

  • Time-, angle- and kinetic-energy-resolved photoelectron spectroscopy of highly excited states of NO, P. Traps, F. Buchner, M. Ghotbi, A. Lubcke, H-H Ritze, M. J. J. Vrakking, A. Rouzee, J. Phys. B, 47, 124016, (2014).

  • Tracing Electron-Ion Recombination in Nanoplasmas Produced by Extreme-Ultraviolet Irradiation of Rare-Gas Clusters, B. Schuette, F. Campi, M. Arbeiter, T. Fennel, M. J. J. Vrakking, A. Rouzee, Phys. Rev. Lett., 112, 253401, (2014).

  • X-ray diffraction from isolated and strongly aligned gas-phase molecules with a free-electron laser, J. Kuepper, S. Stern, L. Holmegaard, F. Filsinger, A. Rouzee, D. Rolles, A. Rudenko, et al., Phys. Rev. Lett., 112, 083002, (2014).

  • Rare-Gas Clusters in Intense Extreme-Ultraviolet Pulses from a High-Order Harmonic Source, B. Schuette, M. Arbeiter, T. Fennel, M. J. J. Vrakking, A. Rouzee, Phys. Rev. Lett., 112, 073003, (2014).

  • Imaging Molecular structure through femtosecond photoelectron diffraction on spatially aligned and oriented gas-phase molecules, R. Boll, A. Rouzee, et al., Faraday discussion, 171, 57, (2014).

  • Formation of coherent rotational wavepackets in small molecule-helium clusters using impulsive alignment, G. Galinis et al., Faraday discussion, 171, 195, (2014).

  • Towards atomic resolution diffractive imaging of isolated molecules with x-ray free electron lasers, S. Stern, L. Holmegaard, F. Filsinger, A. Rouzee, et al., Faraday discussion, 171, 393, (2014).

  • Femtosecond photoelectron diffraction on laser-aligned molecules: Towards time-resolved imaging of molecular structure, R. Boll, et al., Phys. Rev. A, 88, 061402, (2013).

  • Photoelectron imaging of XUV photoionization of CO2 by 13−40 eV synchrotron radiation, F.J. Furch, S. Birkner, J. H. Jungmann, F. Kelkensberg, C. P. Schulz, A. Rouzee, M. J. J. Vrakking, The Journal of chemical physics 139, 124309, (2013).

  • Interference in the angular distribution of photoelectrons in superimposed XUV and optical laser fields, S. Duesterer, L. Rading, P. Johnsson, A. Rouzee, A. Hundertmark, M. J. J. Vrakking, et al., Journal of Physics B, 46, 164026, (2013).

  • Inner-shell multiple ionization of polyatomic molecules with an intense x-ray free-electron laser studied by coincident ion momentum imaging, B. Erk et al., Journal of Physics B, 46, 164031, (2013).

  • Coulomb explosion of diatomic molecules in intense XUV fields mapped by partial covariance, O. Kornilov, M. Eckstein, M. Rosenblatt, C. P. Schulz, K. Motomura, A. Rouzee, et al. Journal of Physics B, 46, 164028, (2013).

  • Photoelectron angular distributions for the two-photon sequential double ionization of xenon by ultrashort extreme ultraviolet free electron laser pulses, S. Mondal et al., Journal of Physics B, 46, 164022, (2013).

  • Towards imaging of ultrafast molecular dynamics using FELs, A. Rouzee, P. Johnsson, L. Rading, A. Hundertmark, W. Siu, Y. Huismans, S. Duesterer, et al., Journal of Physics B, 46, 164029, (2013).

  • Probing Time-Dependent Molecular Dipoles on the Attosecond Time Scale, C. Neidel, J. Klei, CH. Yang, A. Rouzee, M. J. J. Vrakking, K. Kluender, M. Miranda, et al., Physical Review Letters 111, 033001, (2013).

  • Hydrogen Atoms under Magnification: Direct Observation of the Nodal Structure of Stark States, A. S. Stodolna, A. Rouzee, F. Lepine, et al., Physical review letters, 110, 213001, 2, (2013).

  • Single-Size Thermometric Measurements on a Size Distribution of Neutral Fullerenes, C. Cauchy, J. M. Bakker, Y. Huismans, A Rouzee, et al., Physical review letters, 110, 193401, (2013).

  • Photoelectron angular distributions from the ionization of xenon Rydberg states by midinfrared radiation, Y. Huismans, A. Rouzee, et al., Physical Review A, 87, 033413, (2013).

  • Ultrafast Charge Rearrangement and Nuclear Dynamics upon Inner-Shell Multiple Ionization of Small Polyatomic Molecules, B. Erk, et al., Physical review letters, 110, 053003, (2013).

  • Photoelectron angular distributions for the two-photon ionization of helium by ultrashort extreme ultraviolet free-electron laser pulses, R. Ma, K. Motomura, K. L. Ishikawa, S. Mondal, H. Fukuzawa, A. Yamada, K. Ueda, K. Nagaya, S. Yase, Y. Mizoguchi, M. Yao, A. Rouzee, A. Hundermark, M. J. J. Vrakking, P. Johnsson, M. Nagasono, K. Tono, T. Togashi, Y. Senba, H. Ohashi, M. Yabashi and T. Ishikawa, J. Phys. B., 46, 164018, (2013).

  • Scaling Laws for Photoelectron Holography in the Midinfrared Wavelength Regime, Y. Huismans, A. Gijsbertsen, A. S. Smolkowska, J. H. Jungmann, A. Rouzee, et al., Physical Review Letters, 109, 013002, (2012).

  • Photoelectron kinetic and angular distributions for the ionization of aligned molecules using a HHG source, A. Rouzee, F. Kelkensberg, W. K. Siu, G. Gademann, R. R. Lucchese, M. J. J. Vrakking Journal of Physics B, 45, 074016, (2012).

  • X-ray–optical cross-correlator for gas-phase experiments at the Linac Coherent Light Source free-electron laser, S. Schorb, et al., Applied Physics Letters, 100,121107, (2012).

  • Attosecond control of dissociative ionization of O2 molecules, W. Siu, F. Kelkensberg, G. Gademann, A. Rouzee, et al., Physical Review A, 84, 063412, (2011).

  • Doubly resonant three-photon double ionization of Ar atoms induced by an EUV free-electron laser, E. V. Gryzlova, et al., Physical Review A, 84, 063405, (2011).

  • XUV ionization of aligned molecules, F. Kelkensberg, A. Rouzee, et al., Physical Review A, 84, 051404, (2011).

  • Evolutionary optimization of rotational population transfer, A. Rouzee, O. Ghafur, K. Vidma, A. Gijsbertsen, O. M. Shir, T. Back, A. Meijer, W. J. van der Zande, D. Parker, M. J. J. Vrakking, Physical Review A, 84, 033415, (2011).

  • Attosecond control in photoionization of hydrogen molecules, F. Kelkensberg, W. Siu, J. F. Perez-Torres, F. Morales, G. Gademann, A. Rouzee, P. Johnsson, M. Lucchini, F. Calegari, J. L. Sanz-Vicario, F. Martin, M. J. J. Vrakking, Physical Review Letters, 107, 043002, (2011).

  • Angle-resolved photoelectron spectroscopy of sequential three-photon triple ionization of neon at 90.5 eV photon energy, A. Rouzee, et al., Physical Review A, 83, 031401, (2011).

  • Time-resolved holography with photoelectrons, Y. Huismans, A. Rouzee, et al., Science 331, 61, (2011).

  • D2hTDS-ST software for Stark spectrum simulation of X2Y4 asymmetric-top molecules , M Sanzharov, M. Rotger, C. Wenger, M. Loete, V. Boudon, A. Rouzee, Journal of Quantitative Spectroscopy and Radiative Transfer, 112, 41, (2011).

  • Characterization of a two−color pump−probe setup at FLASH using a velocity map imaging spectrometer, P. Johnsson, A. Rouzee, W. Siu, Y. Huismans, F. Lepine, T. Marchenko, S. Duesterer, F. Tavella, N. Stojanovic, A. Azima, R. Treusch, M. F. Kling, M. J. J. Vrakking, Optics letters, 35, 4163, (2010).

  • Non-linear processes in the interaction of atoms and molecules with intense EUV and X-ray fields from SASE free electron lasers (FELs), N. Berrah, et al., Journal of Modern Optics, 57, 1015, (2010).

  • Optimization of laser field-free orientation of a state-selected NO molecular sample, A. Rouzee, A. Gijsbertsen, O. Ghafur, O. M. Shir, T. Back, S. Stolte, M. J. J. Vrakking, New Journal of Physics, 11, 105040, (2009).

  • Field-free molecular alignment probed by the free electron laser in Hamburg (FLASH), P. Johnsson, A. Rouzee, W. Siu, Y. Huismans, F. Lepine, T. Marchenko, S. Duesterer, F. Tavella, N. Stojanovic, A. Azima, R. Treusch, M. F. Kling, M. J. J. Vrakking, Journal of Physics B, 42, 134017, (2009).

  • Impulsive orientation and alignment of quantum-state-selected NO molecules, O. Ghafur, A. Rouzee, A. Gijsbertsen, W. K. Siu, S. Stolte, M. J. J. Vrakking, Nature physics, 5, 289, (2009).

  • Towards the adaptive optimization of field-free molecular alignment, A. Rouzee, E. Hertz, B. Lavorel, O. Faucher, Journal of Physics B, 41, 074002, (2008).

  • Ultimate field-free molecular alignment by combined adiabatic-impulsive field design, S. Guerin, A. Rouzee, E. Hertz, Physical review A, 77, 041404, (2008).

  • Field-free molecular alignment of asymmetric top molecules using elliptically polarized laser pulses, A. Rouzee, S. Guerin, O. Faucher, B. Lavorel, Physical Review A, 77, 043412, (2008).

  • Suppression of plasma contribution in femtosecond degenerate four-wave mixing (fs−DFWM) at high intensity, A. Rouzée, V. Renard, S. Guerin, O. Faucher, B. Lavorel, Journal of Raman Spectroscopy, 38, 969, (2007).

  • Optimization of field-free molecular alignment by phase-shaped laser pulses, E. Hertz, A. Rouzee, S. Guérin, B. Lavorel, O. Faucher, Physical Review A, 75, 031403, (2007).

  • Optical gratings induced by field-free alignment of molecules, A. Rouzee, V. Renard, S. Guerin, O. Faucher, B. Lavorel, Physical Review A, 75, 013419, (2007).

  • Molecular alignment as a calibration method for the determination of ionisation probability,V. Loriot, E. Hertz, A. Rouzee, B. Lavorel, O. Faucher, Journal de Physique IV, 135, 229, (2006).

  • Strong-field molecular ionization: determination of ionization probabilities calibrated with field-free alignment, V. Loriot, E. Hertz, A. Rouzee, B. Sinardet, B. Lavorel, O. Faucher, Optics letters, 31, 2897, (2006).

  • Field-free one-dimensional alignment of ethylene molecule, A. Rouzee, S. Guerin, V. Boudon, B. Lavorel, O. Faucher, Physical Review A, 73, 033418, (2006).

  • Rotational Raman spectroscopy of ethylene using a femtosecond time-resolved pump-probe technique, A. Rouzee, V. Boudon, B. Lavorel, O. Faucher, W. Raballand, The Journal of chemical physics, 123, 154309, (2005).

  • Laser spatial profile effects in measurements of impulsive molecular alignment, A. Rouzee, V. Renard, B. Lavorel, O. Faucher, Journal of Physics B, 38, 2329, (2005).

  • Nonintrusive monitoring and quantitative analysis of strong laser-field-induced impulsive alignment, V. Renard, M. Renard, A. Rouzee, S. Guerin, H-R. Jauslin, B. Lavorel, O. Faucher, Physical Review A, 70, 033420, (2004).

  • Book Chapters:

    • XUV attosecond photoionization and related ultrafast processes in diatomic and large molecules, V. Despre, A. Marciniak, T. Barillot, V. Loriot, A. Rouzee, M. J. J. Vrakking, F. Lepine, Ultrafast Dynamics Driven by Intense Light Pulses, 125-141, (2016).

    • Molecular Movies from Molecular Frame Photoelectron Angular Distribution (MF-PAD) Measurements, A. Rouzee, Y. Huismans, F. Kelkensberg, A. Smolkowska, J.H. Jungmann, et al., Ultrafast Phenomena in Molecular Sciences, 1-24, (2014).

    • Alignment and Orientation of Hexapole State-Selected Molecules, A Rouzee, A Gijsbertsen, M. J. J. Vrakking, Progress in Ultrafast Intense Laser Science VI, 45-73, (2010).